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Reference type: Journal
Authors: Striegler S, Tewes E
Article Title: Investigation of sugar-binding sites in ternary ligand-copper(II)-carbohydrate complexes.
Publication date: 2002
Journal: European Journal of Inorganic Chemistry
Issue: (2)
Page numbers: 487-495.
DOI: 10.1002/1099-0682(20022)2002:2<487::AID-EJIC487>3.0.CO;2-D

Abstract: Evaluation of the binding interactions between a template (such as a carbohydrate) and a functional monomer (such as a metal complex) is one of the key steps during the design of molecularly imprinted polymers. Since we are interested in the development of carbohydrate-imprinted polymers as functional enzyme mimics, we have evaluated the binding interactions of several carbohydrates with [(diethylenetriamine)copper(II)] dinitrate (1), [ N- {(2- hydroxyethyl)ethylenediamine}copper(II)] dichloride (8), and [{4-(N-vinylbenzyl)-diethylenetriamine}copper(II)] diformate (13) in aqueous solution. The binding sites of epimeric carbohydrates in complex formation with different copper(II) complexes have been investigated for the first time. The ternary ligand-copper(II)-carbohydrate complexes produced have been characterized by determination of their stoichiometry and their binding strength, by UV/Vis spectroscopy at alkaline pH

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