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Reference type: Journal
Authors: Rzysko W, Sokolowski S, Pizio O
Article Title: Theory of adsorption in a polydisperse templated porous material: Hard sphere systems.
Publication date: 2002
Journal: Journal of Chemical Physics
Volume: 116
Issue: (10)
Page numbers: 4286-4292.
DOI: 10.1063/1.1450556

Abstract: A theoretical description of adsorption in a templated porous material, formed by an equilibrium quench of a polydisperse fluid composed of matrix and template particles and subsequent removal of the template particles is presented. The approach is based on the solution of the replica Ornstein-Zernike equations with Percus-Yevick and hypernetted chain closures. The method of solution uses expansions of size-dependent correlation functions into Fourier series, as described by Lado [J. Chem. Phys. 108, 6441 (1998)]. Specific calculations have been carried out for model systems, composed of hard spheres. (C) 2002 American Institute of Physics


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