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Reference type: Journal
Authors: Kanekiyo Y, Ono Y, Inoue K, Sano M, Shinkai S
Article Title: "Molecular-imprinting" in polyion complexes which creates the "memory" for the AMP template.
Publication date: 1999
Journal: Journal of the Chemical Society-Perkin Transactions 2
Issue: (3)
Page numbers: 557-561.
DOI: 10.1039/a808117d

Abstract: The formation of a polyion complex precipitate was applied to molecular imprinting for the first time. Polyanion containing boronic acid units can sustain AMP by a boronate-cis-diol interaction. When this polyanion forms a polyion complex with polycation according to 1 : 1 cation-anion stoichiometry,the phosphate anionic charges introduced into the polyanion by the AMP complexation are also counted. Thus, after removal of AMP from the polyion complex a 'cleft' which has the memory for the AMP template is created. It was proved that this cleft shows high affinity with AMP. We also noticed that the removal and re-binding processes for AMP coincide with the swelling and deswelling phenomena of this polyion complex

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