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Reference type: Journal
Authors: Kim YD, Jeon JB, Chang JY
Article Title: CdSe quantum dot-encapsulated molecularly imprinted mesoporous silica particles for fluorescent sensing of bisphenol A.
Publication date: 2012
Journal: Journal of Materials Chemistry
Volume: 22
Issue: (45)
Page numbers: 24075-24080.
DOI: 10.1039/C2JM34798A

Abstract: We prepared a highly sensitive molecularly imprinted fluorescent sensor by using a CdSe quantum dot (QD) as a signal transducer and a mesoporous silica nanoparticle as an imprinting material. Bisphenol-A (BPA) was chosen as a model template, which is known as an endocrine disruptor. Binding sites were selectively formed between the pores and CdSe QDs were encapsulated in the pores of the mesoporous silica. QD-encapsulated, molecularly imprinted mesoporous silica (QD-MIMS) particles exhibited excellent molecular recognition properties in terms of both sensitivity and selectivity. Owing to the proximity of the binding sites to the QDs, a significant, concentration-sensitive fluorescence quenching was observed in the presence of BPA. QD-MIMS showed a linear Stern-Volmer relationship for BPA and its analogs. QD-MIMS had a much larger quenching constant for BPA (by more than ten times) than for BPA analogs, demonstrating the high selectivity of QD-MIMS
Template and target information: bisphenol A, BPA


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