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Reference type: Journal
Authors: Ohkubo K, Sawakuma K, Sagawa T
Article Title: Influence of cross-linking monomer and hydrophobic styrene comonomer on stereoselective esterase activities of polymer catalyst imprinted with a transition-state analogue for hydrolysis of amino acid esters.
Publication date: 2001
Journal: Polymer
Volume: 42
Issue: (5)
Page numbers: 2263-2266.
DOI: 10.1016/S0032-3861(00)00453-5

Abstract: Polymer catalysts, cross-linked with N,N'-ethylene (C-2) {or butylene (C-4)}-bisacrylamide containing L-histidine and quaternary trimethylammonium groups were imprinted with a racemic transition-state analogue of phenyl 1- benzyloxycarbonyl-3-methylpentylphosphonate for the hydrolysis of p-ni(rophenyl N-(benzyloxycarbonyl)-L (or D)-leucinate {Z-L (Dr D)-Leu-PNP}. Maximal stereoselectivity (L/D = 8.4) was obtained by using N,N'-C-4-bisacrylamide cross-linked polymer catalyst, which was copolymerized with hydrophobic styrene monomer. (C) 2000 Elsevier Science Ltd. All rights reserved


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