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Reference type: Journal
Authors: Dai YL, Li XY, Fan LM, Lu XJ, Kan XW
Article Title: "Sign-on/off" sensing interface design and fabrication for propyl gallate recognition and sensitive detection.
Publication date: 2016
Journal: Biosensors and Bioelectronics
Volume: 86
Page numbers: 741-747.
DOI: 10.1016/j.bios.2016.07.072
Alternative URL: http://www.sciencedirect.com/science/article/pii/S095656631630700X

Abstract: A new strategy based on sign-on and sign-off was proposed for propyl gallate (PG) determination by an electrochemical sensor. The successively modified poly(thionine) (PTH) and molecular imprinted polymer (MIP) showed an obvious electrocatalysis and a good recognition toward PG, respectively. Furthermore, the rebound PG molecules in imprinted cavities not only were oxidized but also blocked the electron transmission channels for PTH redox. Thus, a sign-on from PG current and a sign-off from PTH current were combined as a dual-sign for PG detection. Meanwhile, the modified MIP endowed the sensor with recognition capacity. The electrochemical experimental results demonstrated that the prepared sensor possessed good selectivity and high sensitivity. A linear ranging from 5.0 x 10-8 to 1.0 x 10-4 mol/L for PG detection was obtained with a limit of detection of 2.4 x 10-8 mol/L. And the sensor has been applied to analyze PG in real samples with satisfactory results. The simple, low cost, and effective strategy reported here can be further used to prepare electrochemical sensors for other compounds selective recognition and sensitive detection
Template and target information: propyl gallate, PG
Author keywords: Electrochemical sensor, Propyl gallate, molecular imprinted polymer, Poly(thionine), Dual-sign


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