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Reference type: Journal
Authors: Jiang HM, Zhang YD, Chen RN, Sun ML, Tong HY, Xu JY
Article Title: Preparation of ion imprinted magnetic Fe3O4 nanoparticles for selective remediation of Pb(II).
Publication date: 2017
Journal: Journal of the Taiwan Institute of Chemical Engineers
Volume: 80
Page numbers: 184-191.
DOI: 10.1016/j.jtice.2017.06.047
Alternative URL: http://www.sciencedirect.com/science/article/pii/S1876107017303425

Abstract: A novel Pb(II) imprinted magnetic polymer (Pb-IIMP) was synthesized by surface imprinting technique using Pb(II) as template, polyethyleneimine functionalized magnetic Fe3O4 (MNPs@PEI) as functional monomer and epoxy chloropropane (ECH) as cross-linker and applied for the remediation of Pb(II). Batch adsorption studies were performed to evaluate the influence of different sorption parameters, such as pH, initial concentration of Pb(II), contact time, adsorption selectivity and desorption. Isotherm and kinetics studies showed that the adsorption process obeyed Langmuir and pseudo-second-order models with a maximum adsorption capacity of 123.3 mg/g for Pb-IIMP and 62.2 mg/g for non-imprinted magnetic polymer (Pb-NIMP). The relative selectivity coefficients of Pb-IIMP for Pb(II)/Cd(II) and Pb(II)/Cu(II) were 1.2 and 1.4 times greater than Pb-NIMP. In addition, Pb(II) could be desorbed from Pb-IIMP by 0.5 mol/L HCl and used for five cycles without any adsorption performance loss, which revealed that the prepared Pb-IIMP had high stability and good reusability
Template and target information: lead ion, Pb(II)
Author keywords: Ion imprinted magnetic polymer, Surface imprinted technique, Pb(II), adsorption


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