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Reference type: Journal
Authors: Sun Y, Feng XW, Hu J, Bo S, Zhang JM, Wang W, Li SY, Yang YF
Article Title: Preparation of hemoglobin (Hb)-imprinted poly(ionic liquid)s via Hb-catalyzed eATRP on gold nanodendrites.
Publication date: 2020
Journal: Analytical and Bioanalytical Chemistry
Volume: 412
Issue: (4)
Page numbers: 983-991.
DOI: 10.1007/s00216-019-02324-w

Abstract: Hemoglobin (Hb)-imprinted poly(ionic liquid)s (HIPILs) were prepared on the surface of Au electrode modified with gold nanodendrites (Au/ND/HIPILs). HIPILs were synthesized with 1-vinyl-3-propyl imidazole sulfonate ionic liquids as functional monomers via electrochemically mediated atom transfer radical polymerization (eATRP) catalyzed by Hb. The Au/ND/HIPILs electrode was examined by cyclic voltammetry (CV), scanning electron microscope (SEM), and X-ray photoelectron spectroscopy (XPS). The Au/ND/HIPILs electrode was also used as an electrochemical sensor to determine Hb by differential pulse voltammetry (DPV). Under the optimal conditions, the detection range of Hb was from 1.0 × 10-14 to 1.0 × 10-4 mg/mL with a limit of detection of 5.22 × 10-15 mg/mL (S/N = 3). Compared with other methods, the sensor based on poly(ionic liquid)s had the broader linear range and lower detection limit
Template and target information: protein, hemoglobin, Hb
Author keywords: Superoxide dismutase, Poly(ionic liquid)s, Electrochemically mediated atom transfer radical polymerization

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