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Reference type: Journal
Authors: Rosengren AM, Karlsson BCG, Nicholls IA
Article Title: Consequences of Morphology on Molecularly Imprinted Polymer-Ligand Recognition.
Publication date: 2013
Journal: International Journal of Molecular Sciences
Volume: 14
Issue: (1)
Page numbers: 1207-1217.
DOI: 10.3390/ijms14011207

Abstract: The relationship between molecularly imprinted polymer (MIP) morphology and template-rebinding over a series of warfarin-imprinted methacrylic acid co(ethylene dimethacrylate) polymers has been explored. Detailed investigations of the nature of template recognition revealed that an optimal template binding was obtained with polymers possessing a narrow population of pores (~3-4 nm) in the mesopore size range. Importantly, the warfarin-polymer rebinding analyses suggest strategies for regulating ligand binding capacity and specificity through variation of the degree of cross-linking, where polymers prepared with a lower degree of cross-linking afford higher capacity though non-specific in character. In contrast, the co-existence of specific and non-specific binding was found in conjunction with higher degrees of cross-linking and resultant meso- and macropore size distributions.
Template and target information: warfarin
Author keywords: molecularly imprinted polymer, MIP, morphology, BET, Surface area, Warfarin


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